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Ok I couldn't think of my absolute favorite and it tied between these two.

Kingdom Hearts 2 Twilight Town Battle Theme (Don't know the name)
http://www.youtube.com/watch?v=VsGPV_FgHX4

But quite honestly, could be most of the music in KH (Except mabye the TLM ones xD)

and....

Tobli from Golden Sun
http://www.youtube.com/watch?v=8Om1m_WlORY

It's so damn relaxing, I could listen for hours.

Rayman 2 Sanctuary of water and ice: http://www.youtube.com/watch?v=JVRYDJO1wes It just builds to epicness, and it's good music to listen to even if you're just doing some kind of work, and this:
Halo 3 never forget: http://www.youtube.com/watch?v=d7w76B7fO_4 Is sad and uplifting at the same time.

Favourite songs,no particular order.

Portal - Still Alive
http://www.youtube.com/watch?v=Y6ljFaKRTrI

Portal 2 - Want You Gone
http://www.youtube.com/watch?v=dVVZaZ8yO...ure=fvwrel

Fallout 3 - I Don't Want To Set The World On Fire
http://www.youtube.com/watch?v=n9D6GNzpmkM

Fallout: New Vegas - Jonhy Guitar
http://www.youtube.com/watch?v=V2VTulxEDig

Fallout: New Vegas - Let's Ride Into the Sunset Together
http://www.youtube.com/watch?v=k9N9cffFu...ure=relmfu

...and some more.

inFamous 2 - Fade Away
http://www.youtube.com/watch?v=VDjovrzqDJM